- Bleecker Street (Demo 1964)
- The Sound Of Silence (acoustic version)
- The Sun Is Burning
- Wednesday Morning, 3 A.M.
- He Was My Brother
- Sparrow
- Peggy-O
- Benedictus
- Somewhere They Can't Find Me
- We've Got A Groovy Thing Goin'
- Leaves That Are Green
- Richard Cory
- I Am A Rock
- The Sound Of Silence (Electric version)
- Homeward Bound
- Blues Run The Game (Studio Outtake - 1965)
- Kathy's Song
- April Come She Will
- Flowers Never Bend With The Rainfall
- Patterns
- Cloudy
- The Dangling Conversation
- Scarborough Fair/Canticle
- The 59th Street Bridge Song (Feelin' Groovy)
- For Emily, Whenever I May Find Her
- 7 O'clock News/Silent Night
- A Hazy Shade Of Winter
- At The Zoo
- A Poem On The Underground Wall (live At Lincoln Center, New York City, NY - January 1967)
- Red Rubber Ball (live At Lincoln Center, New York City, NY - January 1967)
- Blessed (live At Lincoln Center, New York City, NY - January 1967)
- Anji (live At Lincoln Center, New York City, NY - January 1967)
- A Church Is Burning (live At Lincoln Center, New York City, NY - January 1967)
- Fakin' It
- Save The Life Of My Child
- America
- You Don't Know Where Your Interest Lies (single B-Side - 1968)
- Punky's Dilemma
- Comfort & Joy
- Star Carol
- Mrs. Robinson
- Old Friends/Bookends (single mix)
- Overs (live At Memorial Auditorium, Burlington, VT - October 1968)
- A Most Peculiar Man (live At Memorial Auditorium, Burlington, VT - October 1968)
- Bye Bye Love (live At Memorial Auditorium, Burlington, VT - October 1968)
- The Boxer
- Baby Driver
- Why Don't You Write Me
- Feuilles-O (Demo - 1969)
- Keep The Customer Satisfied
- So Long, Frank Lloyd Wright
- Song For The Asking
- Cecilia
- El Condor Pasa
- Bridge Over Troubled Water
- The Only Living Boy In New York
- Hey Schoolgirl/Black Slacks (live At Carnegie Hall, New York, NY - November 1969)
- That Silver Haired Daddy Of Mine (live At Carnegie Hall, New York, NY - November 1969)
- My Little Town
| 59 tracks | Legacy/Columbia |
